Compared to the “ideal IR LED” by cerupcat and a few others - scroll down on this page - http://nuigroup.com/forums/viewthread/2694/P0/ - its half-angle seems to be on the low side. The minimum half angle should be at least +/- 48 degrees, but your LEDs are +/- 13 degrees according to the data sheet. “Anything less than +/- 48 will not take full advantage of TIR”.