It seems that the main reason you have for adding more IR illuminators is poor finger-tracking illumination.
Perhaps your setup might benefit from a combination DI/FITR setup. DI gives you even lighting for fiducials, however, FTIR gives superior blob performance. Since you are using a compliant surface anyhow (rather than attaching your screen material to the underside surface), perhaps you could illuminate the acrylic edge-on with strip-LED lighting, then place your Rosco grey over a compliant surface (or even silicone coat the bottom of your roscoe).
In this way you could get good finger tracking. It shouldn’t take much IR lighting to light the Fiducials (it seems that it is more important to have them evenly lit than brightly lit), probably a lot fewer LEDs than you already have in your arrays. Considering that you should get some illumination from the edge-on IRs, I bet you could get away with as few as 10 or 20 illuminating LEDs projecting to the bottom of the screen.
It seems that the major advantage of a DI (or DRI) setup is
1) having your fingers on glass rather than a compliant surface, and mounting the projection material on the underside vs acrylic covered with a damagable surface (FTIR). and
2) Fiducial/Symbol recognition.
Considering you are already using a projection material on your top surface this seems to be the ideal situation for a hybrid DRI/FTIR setup.
I am inspired by your DI project and hope to try a hybrid DRI/FTIR setup myself now....